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Title | Phonon density of states in epitaxial Fe/Cr(001) superlattices |
Creator/Author | Ruckert, T. ; Keune, W. ; Sturhahn, W. ; Hu, M. Y. ; Sutter, J. P. ; Toellner, T. S. ; Alp, E. E. |
Publication Date | 1999 Oct 21 |
OSTI Identifier | OSTI ID: 750539 |
Report Number(s) | ANL/XFD/CP-100200 |
DOE Contract Number | W-31109-ENG-38 |
Other Number(s) | TRN: AH200020%%164 |
Resource Type | Conference |
Resource Relation | Conference: International Conference on Applications of the Moessbauer Effect 1999, Garmisch-Partenkirchen (DE), 08/29/1999--09/03/1999; Other Information: PBD: 21 Oct 1999 |
Research Org | Argonne National Lab., IL (US) |
Sponsoring Org | US Department of Energy (US) |
Subject | 36 MATERIALS SCIENCE; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; IRON; CHROMIUM; SUPERLATTICES; LAYERS; PHONONS; LATTICE VIBRATIONS; IRON 57; IRON ALLOYS; CHROMIUM BASE ALLOYS; MOESSBAUER EFFECT |
Description/Abstract | Incoherent nuclear resonant absorption of synchrotron radiation at the 14.413 keV nuclear resonance of {sup 57}Fe was employed to measure directly the Fe-projected (partial) photon density of states (DOS) in epitaxial [Fe(8.7ML)/Cr(8ML)]{sub 200} superlattices and alloy films MBE-grown on MgO(001). Isotopically depleted {sup 56}Fe was used which gives no resonance signal. 0.7 monolayers (ML) thick {sup 57}Fe-probe layer (1{angstrom}) of 95.5% enrichment were placed either at the {sup 56}Fe-on-Cr interfaces or at the center of the {sup 56}Fe layers, thus providing a nuclear resonance signal from different places in the films. In addition, the authors prepared an epitaxial film which contains only a 1{angstrom}-thick {sup 57}Fe submonolayer in Cr(001) and no {sup 56}Fe layers. Moreover, they prepared a 7000 {angstrom}-thick epitaxial {sup 57}Fe{sub 0.03}Cr{sub 0.97}(001) alloy film. The measurements were performed at 300 K with 2.3 meV energy resolution around 14.413 keV. The phonon DOS of the center site was found to be very similar to that of bulk bcc Fe. Compared to the center site, the DOS of the other samples show distinct differences. In particular, longitudinal vibrations of Fe atoms are suppressed at the Fe/Cr interfaces. |
Country of Publication | United States |
Language | English |
Format | Medium: P; Size: 10 pages |
Availability | INIS; OSTI as DE00750539 To purchase this media from NTIS, click here |
System Entry Date | 2008 Feb 05 |
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