1. Introduction
EMSL Research
Research Capabilities
Accessing the EMSL
Mission
Research Overview
2. Oxide Films and Surfaces
Development of a Novel Deposition Method for Synthesis of Porous Oxide Thin Films(a)
Y. Gao and S. Elder
X-Ray Photoelectron Diffraction of MgO(111)-(1x1)(b,c)
M. Gajdardziska-Josifovska, R. Plass, and S. A. Chambers
Low-Energy Cathodoluminescence Spectroscopy of Al-Doped TiO2 Films(b,d)
S. Goss, L. J. Brillson, and S. A. Chambers
Surface Termination and Interlayer Relaxations in Fe3O4(001)(b-g)
S. A. Chambers, S. Thevuthasan, S. A. Joyce, B. Stanka, W. Hebenstreit, and U. Diebold
Lattice Mismatched Oxide Heteroepitaxy – a
-Fe2O3/a
-Al2O3(0001)(b,d)
S. I. Yi, Y. Liang, S. Thevuthasan, D. E. McCready, and S. A. Chambers
Reaction of Water with Well-Defined Iron Oxide Surfaces(b-e,h)
P. Liu, E. Nelson, T. Kendelewicz, G. E. Brown, Jr., Y. J. Kim, and S. A. Chambers
Redox Chemistry of Chromate with Well-Defined Iron Oxide Surfaces(b-e,h)
P. Liu, C. Doyle, E. Nelson, T. Kendelewicz, G. E. Brown, Jr., and S. A. Chambers
Cleaving Oxide Films Using Hydrogen Implantation(b,d,e)
S. Thevuthasan, W. Jiang, and W. J. Weber
3. Nanoscale Materials
Spatially Designed Molecular Monolayers in Ordered Nanoscale Materials(d,i)
J. Liu, G. E. Fryxell, L.-Q. Wang, Y. Shin, G. J. Exarhos, and S. Baskaran
Nanoscale Fabrication for Enhanced Properties(a)
D. R. Baer and Y. Liang
Dense Arrays of Well-Aligned Carbon Nanotube Thin Films(a,b,d)
Y. Gao, J. Liu, M. Shi, S. H. Elder, and J. W. Virden
Quantum Dot Molecules(b)
M. H. Na, H. Luo, and Y. Liang
4. Electronic Materials
Effectiveness of High Energy Ion Beam Techniques for the Characterization of Mesoporous Low Dielectric-Constant Materials(b,j)
S. Baskaran, J. Liu, and S. Thevuthasan
Effects of Precursors and Substrate Materials on Microstructure, Dielectric Properties and Step Coverage of (Ba,Sr)TiO3 Films Grown by Metalorganic Chemical Vapor Deposition(b,k)
Y. Gao, S. He, M. Engelhard, A. S. Lea, P. Alluri, J. Finder, B. Melnick, and R. L. Hance
Mechanistic Study of Metalorganic Chemical Vapor Deposition of (Ba,Sr)TiO3 Thin Films(b,j,k)
Y. Gao, C. L. Perkins, S. He, T. Tran, S. Thevuthasan, M. A. Henderson, P. Alluri, and T. Baum
Interplay Between Interfacial Properties and Dielectric and Ferroelectric Behaviors of Barium Strontium Titanate Thin Films(j)
Y. Liang, S. A. Chambers, S. Gan, and D. R. Baer
Development of Low-Temperature ITO Process for Flat Panel Display(l)
P. M. Martin and G. L. Graff
5. Separation Processing and Materials
Molecular Design of Agents for Selective Anion Separation(m)
T. L. Hubler, J. H. Sukamto, G. M. Anderson, S. A. Bryan, G. J. Lumetta
Electroactive Materials for Anion Separation—Technetium from Nitrate(e)
J. P. H. Sukamto, S. D. Rassat, T. L. Hubler, M. A. Lilga, G. M. Anderson, S. A. Bryan, W. H. Smyrl, and J. McBreen
Electrically Switched Ion Exchange (ESIX) for the Separation of Potassium and Chloride Ions to Enhance Water Recycle(n)
J. P. H. Sukamto, S. D. Rassat, W. E. Lawrence, G. B. Josephson, V. V. Viswanathan, D. P. Mendoza, A. S. Lea, J. S. Young, R. T. Hallen, R. J. Orth, W. A. Wilcox, M. A. Lilga, S. A. Bryan, B. J. Malmberg, Y. Gu, L. L. Edwards, and P. Thorn
6. Interfacial Properties and Reactivity
Development of Novel Photocatalysts Using Interfacial Engineering(a)
Y. Liang, J. L. Daschbach, S. A. Chambers, Y. Su, Y. Wang, H. Luo, and S. Gan
Local Reactions on Carbonate Surfaces: Structure, Reactivity and Solution(d)
D. R. Baer, J. E. Amonette, Y. Liang, A. S. Lea, L. Sorenson, and P. Geissbuhler
Ion-Channeling Study of the SiC/Si/SiO2/Si Interface(b,d)
W. Jiang, F. Namavar, S. Thevuthasan, and W. J. Weber
Investigation of Hematite Film-Substrate Interfaces Using Rutherford Backscattering and Channeling Techniques(b-e,o)
S. Maheswaran, R. J. Smith, S. Thevuthasan, and S. A. Chambers
Selected Functionalization of Polymer Surfaces by Plasma-Immobilization of Functional Molecules(a,p)
M. K. Shi, X. Y. Gong, G. L. Graff, J. D. Affinito, and G. J. Exarhos
Fundamentals of Stress Corrosion Cracking: Light-Weight Materials Influence of Mg on the Corrosion of Al(d)
D. R. Baer, C. F. Windisch, Jr., M. H. Engelhard, M. J. Danielson, R. H. Jones, and J. S. Vetrano
7. Catalysis
Ionizing Radiation Induced Catalysis on Metal Oxide Particles(e)
M. A. Henderson, S. A. Chambers, Y. Su, J. L. Daschbach, Y. Wang, C. H. F. Peden, C. L. Perkins, Prof. M. E. Castro, Prof. A. K. Datye, Prof. J. Osterwalder
Detailed Investigations on Hydrogen Formation by the Photocatalytic Splitting of Water(a)
G. S. Herman, Y. Gao, J. Osterwalder, C. S. Fadley, C. H. F. Peden, M. R. Sievers, and C. L. Perkins
Mesoporous Silica Supported Solid Acid Catalysts(j)
S. Choi, Y. Wang, and C. H. F. Peden
Model Studies of Automobile Exhaust Catalysis Using Single Crystals of Rhodium and Ceria/Zirconia(d)
C. H. F. Peden, G. S. Herman, and D. N. Belton
Plasma Assisted Catalysis(q)
M. L. Balmer, R. Tonkyn, G. Maupin, S. Barlow, S. Yoon, and A. Kolwaite
Plasma Assisted Catalysis for Heavy Duty Diesel Engines(q,r)
C. Habeger, C. Aardahl, and M. L. Balmer
8. Analysis and Measurement
DNA Sample Preparation and Detection for Complex Sample Matrices(a,j)
C. Bruckner-Lea, D. Holman, L. Olson, J. Grate, D. Chandler, M. Stottlemyre, J. Brown, B. Schuck, J. Nielsen, D. Call, E. Jutras, D. Weaver, F. Brockman, J. Price, J. Follansbee, D. St. Pierre, L. Bond, T. Tsukuda, M. Kingsley 8-1
Chemical Analysis by Laser Ablation Mass Spectroscopy(b,e,s)
M. L. Alexander, A. L. Hedges, S. C. Langford, J. T. Dickinson, G. Cardell, and M. Taylor
9. Analysis and Measurement
New Silicotitanate Waste Forms: Development and Characterization(e)
M. L. Balmer, Y. Su, E. Bitten, A. Navrotsky, H. Xu, T. Nenoff, M. Nyman, and R. Roth
Heavy-Ion Irradiation Effects in Pyrochlore Structures for the Immobilization of Actinide-Rich Wastes(e)
B. D. Begg, W. J. Weber, J. P. Icenhower, and S. Thevuthasan
Ion Exchange Processes and Mechanisms in Glasses(e)
B. P. McGrail, D. R. Baer, J. G. Darab, M. H. Engelhard, J. P. Icenhower, D. K. Shuh, S. Thevusathan
Quantification of Water-Content of Simulated Nuclear Waste Glasses Using Nuclear Reaction Measurements(a)
S. K. Sundaram, S. Thevuthasan, and D. E. McCready
Kinetics of Irradiation-Damage Processes in (6H) SiC(d)
W. J. Weber, W. Jiang, and S. Thevuthasan
Accumulation and Recovery of Irradiation Effects in SrTiO3(d)
W. J. Weber, W. Jiang, and S. Thevuthasan
Effect of Oxygen Ion Implantation in Gallium Nitride(d)
W. Jiang, W. J. Weber, and S. Thevuthasan
10. Appendix
Interfacial and Processing Sciences Staff
Publications and Presentations
Publications
In-Press
Patents and Inventions
Presentations
Honors and Recognition
Acronyms and Abbreviations
Where I&PS Fits in PNNL
Funding Support
(a) Pacific Northwest National Laboratory (PNNL) Laboratory Directed Research and Development (LDRD).
(b) EMSL Operations, supported by DOE Office of Biological and Environmental Research (OBER).
(c) National Science Foundation.
(d) DOE Office of Basic Energy Sciences (BES), Materials Sciences Division.
(e) DOE Environmental Management Science Program (EMSP).
(f) National Science Foundation, Faculty Early Career Development.
(g) DOE-Experimental Program to Stimulate Competitive Research (EPSCoR).
(h) National Science Foundation, Materials Research Science and Engineering Center (MRSEC).
(i) U.S. Department of Agriculture.
(j) Laboratory Technology Research (LTR) Program.
(k) Motorola, Inc.
(l) Defense Advanced Research Projects Agency (DARPA).
(m) Laboratory Directed Research and Development funding (STEP Initiative).
(n) DOE Office of Industrial Technologies, Industry of the Future Program, Forest Products.
(o) University of Western Sydney (UWS) Nepean Staff Development Fund.
(p) Environmental and Health Sciences Division (EHSD).
(q) DOE Energy Efficiency Office of Advanced Automotive Technology.
(r) Cooperative Research and Development Agreement (CRADA).
(s) National Aeronautics and Space Administration (NASA).
William R. Wiley Environmental Molecular Sciences Laboratory
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