PUBLIC HEALTH ASSESSMENT
PUBLIC HEALTH IMPLICATIONS OF RADIATION CONTAMINATION AT
FORMER CLOCK FACTORIES LOCATED IN
BRISTOL (HARTFORD COUNTY), NEW HAVEN (NEW HAVEN COUNTY), THOMASTON (LITCHFIELD
COUNTY), AND WATERBURY (NEW HAVEN COUNTY)
CONNECTICUT
Radiation Surveys
Radiation surveys included gamma, alpha, beta radiation, and radon gas sampling. The gamma radiation measurements included direct contact, and waist level or general area readings. The waist level readings are measured at three feet from the suspected source.
The alpha and beta radiation measurements were reported as either fixed or smearable. The smearable results indicate that radioactive contamination is present. The units of radiation are dependent on the radiation type and measurement techniques. Gamma radiation is generally reported in uR/hr (micro Roentgen per hour). Alpha and beta radiation units are either reported as counts per minute (cpm) or disintegrations per minute (dpm). The value of dpm will always be greater than the value for counts per minute, since the efficiency for the alpha detector is approximately 30 percent and the beta/gamma detector is approximately 10 percent. Radon is a radioactive gas that is a decay product of radium. The units of measurement are pCi/L (pico Curie per liter).
The CT DEP requested radiological assistance from the US Department of Energy (DOE) on April 1, 1998. Surveying was conducted from April 2, 1998, to April 7, 1998.
On April 2, 1998, the DOE/CT DEP team conducted sampling at the Waterbury Clock Company including, the Ville Swiss Automatics and Belco.
On April 3, 1998, the investigation proceeded to the former Lux Clock Company in Waterbury.
On April 6, 1998, the radiation survey investigated the former Seth Thomas Clock company in Thomaston, as well as the former Benrus Clock Company in Waterbury.
On April 7, 1998, the Thomaston radiation survey was completed, and a separate survey was conducted in New Haven.
The results of the radiation surveys are presented below in Tables 2 through 14. Each table identifies the town name, former clock company name, current occupant, location of sample, maximum radiation levels detected, background levels, and the relevant comparison value. In 1997, EPA issued OSWER Directive 9200.4-18, Establishment of cleanup levels for Superfund sites with radioactive contamination. This directive provides guidance for establishing protective cleanup levels for radioactive contamination at Superfund sites. Using this directive, an effective dose of 15 mRem/yr equates to an increased lifetime risk of 3 in 10,000 of cancer, serving as the upper bounds of EPA acceptable risk. This would include exposures from all pathways, and through all media (e.g., soil, ground water, surface water, sediment, air, structures, biota).
Table 2. Town: Bristol
Clock Company Name: Sessions Clock Company
Current
Occupant(s): DABKO CO.
Radiological Parameter (units) |
Location | Floor | Measurement Description |
Maximum Level |
Background | CL |
Gamma radiation (uR/hr) |
Building A | 2nd floor | not applicable | 0 | NR | 15 |
3rd floor | not applicable | 0 | ||||
4th floor | not specified | 120 | ||||
Building D | 2nd floor | not applicable | 0 | NR | NR | |
3rd floor | not specified | 40 |
CL = EPA Cleanup Level
NR = not reported
uR/hr = Micro
Roentgen per hour
Table 3. Town: Bristol
Clock Company Name: Sessions Clock Company
Current
Occupant(s): Bristol Instrument Gears
Radiological Parameter (units) |
Location | Measurement Description |
Maximum Level | Background | CL |
Gamma radiation (uR/hr) |
1st floor | Direct contact | 15 | 5 | 15 |
Measured at Waist level | 12 | ||||
Alpha, Beta gamma activity | not measured |
CL = EPA Cleanup Level
uR/hr = Micro
Roentgen per hour
Table 4. Town: New Haven
Clock Company Name: New Haven Clock
Company
Current Occupant(s): Goodies
Repairs
Radiological Parameter (units) | Location | Measurement Description | Maximum Level | Background | CL |
Gamma radiation (uR/hr) | 1st floor | Direct contact | 35 | 10 | 15 |
Measured at Waist level | 13 | ||||
Alpha, Beta gamma activity | not measured |
CL = EPA Cleanup Level
uR/hr = Micro
Roentgen per hour
Table 5. Town: Thomaston
Clock Company Name: Seth Thomas Clock
Company
Current Occupant(s): Various Companies
Radiological Parameter (units) | Location | Measurement Description | Maximum Level | Background | CL |
Gamma radiation (uR/hr) | 1st floor | Direct contact | 100 | 12 | 15 |
General Area | 40 | ||||
2nd floor | Direct contact | 80 | |||
General Area | 25 | ||||
3rd floor | Direct contact | 650 | |||
General Area | 80 | ||||
4th floor | Direct contact | 45 | |||
General Area | 12 | ||||
Alpha activity (net cpm)
DP (cpm/100 cm2) DP (cpm/100 cm2) DP (cpm/100 cm2) DP (cpm/100 cm2) |
1st floor | Fixed | 0 | 0 | 300 20* |
Measurement of Loose Material (Smear) | 0 | 0 | |||
2nd floor | Fixed | not measured | NR | 300 20 |
|
Measurement of Loose Material (Smear) | 0 | 0 | |||
3rd floor | Fixed | 100 | 0 | 300 20 |
|
Measurement of Loose Material (Smear) | 10 | 0 | |||
4th floor | Fixed | 550 | 0 | 300 20 |
|
Measurement of Loose Material (Smear) | 50 | 0 | |||
Beta Gamma activity (net cpm)
DP (cpm/100 cm2) DP (cpm/100 cm2) DP (cpm/100 cm2) DP (cpm/100 cm2) |
1st floor | Fixed | 6,000 | 50 | 300 20 |
Measurement of Loose Material (Smear) | 0 | 50 | |||
2nd floor | Fixed | 500 | 50 | 300 20 |
|
Measurement of Loose Material (Smear) | 0 | 0 | |||
3rd floor | Fixed | 3,000 | 50 | 300 20 |
|
Measurement of Loose Material (Smear) | 30 | 50 | |||
4th floor | Fixed | 1,300 | 50 | 300 20 |
|
Measurement of Loose Material (Smear) | 30 | 50 |
CL = EPA Cleanup Level
cpm = counts per minute
dpm = disintegrations per minute
NR = not reported, background counting rates ranged from 0.2-0.3 cpm for alpha,
and 30-50 cpm for beta/gamma.
uR/hr = Micro Roentgen per hour
*The cpm units can be converted into dpm units, however the calibration isotope
is required for this. In general, if an unconverted cpm value exceeds the dpm
cleanup level, then the converted value will also be greater.
Table 6. Town: Waterbury
Clock Company Name: Benrus Clock Company
Current Occupant(s): Bender Plumbing
Radiological Parameters (units) | Location | Measurement Description | Maximum Level | Background | CL |
Gamma radiation (uR/hr) | 1st floor | Direct contact | 0 | 10 | 15 |
Measured at Waist level | 0 | ||||
2nd floor | Direct contact | 0 | |||
Measured at Waist level | 0 | ||||
3rd floor | Direct contact | 0 | |||
Measured at Waist level | 0 | ||||
4th floor | Direct contact | 120 | |||
Measured at Waist level | 26 | ||||
5th floor | Direct contact | 40 | |||
Measured at Waist level | 15 | ||||
6th floor | Direct contact | 0 | |||
Measured at Waist level | 0 | ||||
7th floor | Direct contact | 600 | |||
Measured at Waist level | 100 | ||||
Radon-222 (pCi/L) | 4th floor | Not applicable | 1.0 | NR | 4 |
CL = EPA Cleanup Level
NR = not reported
pCi/L = Pico Curries per Liter
uR/hr
= Micro Roentgen per hour
Table 7. Town: Waterbury
Clock Company Name: Lux Clock Company
Current Occupant(s): Anchor Advanced Products
Radiological Parameters (units) | Location | Measurement Description | Maximum Level | Background | CL |
Gamma radiation (uR/hr) | 1st floor | Direct contact | 20 | 10 | 15 |
2nd floor | Direct contact | 20 | |||
3rd floor | Direct contact | 30 | |||
4th floor | Direct contact | 140 | |||
Alpha Beta activity(dpm) | 1st floor | Measurement of Loose Material (Smear) | not measured | NR | 20 |
2nd floor | Measurement of Loose Material (Smear) | not measured | NR | ||
3rd floor | Measurement of Loose Material (Smear) | not measured | NR | ||
4th floor | Measurement of Loose Material (Smear) | 150 | NR |
CL = EPA Cleanup Level
dpm = disintegrations per minute
NR= not reported, background counting rates ranged from
0.2-0.3 cpm for alpha, and 30-50 cpm for beta/gamma.
uR/hr
= Micro Roentgen per hour
Table 8. Town: Waterbury
Clock Company Name: Waterbury Clock
Company
Current Occupant(s): Belco 2nd
floor
Radiological Parameter (units) | Location | Measurement Description | Maximum Level | Background | CL |
Gamma radiation (uR/hr) | Cutting Room | Direct contact | 55 | 10 | 15 |
Measured at Waist level | 55 | ||||
Machine Room | Direct contact | 140 | |||
Measured at Waist level | 140 | ||||
Alpha activity(dpm/100 cm2) | Cutting Room | Measurement of Loose Material (Smear) | <MDA | NR | 20 |
Machine Room | Measurement of Loose Material (Smear) | 150 | NR | ||
Beta Gamma activity(dpm/100 cm2) | Cutting Room | Measurement of Loose Material (Smear) | <MDA | NR | 20 |
Machine Room | Measurement of Loose Material (Smear) | 232 | NR |
<MDA = less than minimum detected activity
CL = EPA Cleanup Level
dpm = disintegrations per minute
NR = not reported, background counting rates ranged from
0.2-0.3 cpm for alpha, and 30-50 cpm for beta/gamma.
uR/hr
= Micro Roentgen per hour
Table 9. Town: Waterbury
Clock Company Name: Waterbury Clock
Company
Current Occupant(s): Belco 3rd
floor Highest radiation level detected
Radiological Parameter (units) | Location | Measurement Description | Maximum Level | Background | CL |
Gamma radiation (uR/hr) | Hallway | Direct contact | 5,000 | 10 | 15 |
Measured at Waist level | 1,500 | ||||
Store room | Direct contact | 3,200 | |||
Measured at Waist level | 250 | ||||
Liba room | Direct contact | 300 | |||
Measured at Waist level | 52 | ||||
Alpha activity (dpm/100 cm2) | Hallway | Measurement of Loose Material (Smear) | 7,985 | NR | 20 |
Store room | Measurement of Loose Material (Smear) | 4,438 | NR | ||
Liba room | Measurement of Loose Material (Smear) | 328 | NR | ||
Beta Gamma activity (dpm/100 cm2) | Hallway | Measurement of Loose Material (Smear) | 16,636 | NR | 20 |
Store room | Measurement of Loose Material (Smear) | 9,242 | NR | ||
Liba room | Measurement of Loose Material (Smear) | 695 | NR |
CL = EPA Cleanup Level
dpm = disintegrations per minute
NR = not reported, background counting rates ranged from
0.2-0.3 cpm for alpha, and 30-50 cpm for beta/gamma.
uR/hr
= Micro Roentgen per hour
Table 10. Town: Waterbury
Clock Company Name: Waterbury Clock
Company
Current Occupant(s): Belco 4th
floor
Radiological Parameter (units) | Location | Measurement Description | Maximum Level | Background | CL |
Gamma radiation (uR/hr) | Store room | Direct contact | 120 | 10 | 15 |
Measured at Waist level | 70 | ||||
Radon-222 (pCi/L) | 4th floor | not applicable | 6.5 | NR | 4 |
Alpha activity (dpm/100 cm2) | Store room | Measurement of Loose Material (Smear) | 19 | NR | 20 |
Beta Gamma activity (dpm/100cm2) | Store room | Measurement of Loose Material (Smear) | <MDA | NR | 20 |
CL = EPA Cleanup Level
dpm = disintegrations per minute
NR = not reported, background counting rates ranged from
0.2-0.3 cpm for alpha, and 30-50 cpm for beta/gamma.
pCi/L = Pico Curries per Liter
uR/hr
= Micro Roentgen per hour
Table 11. Town: Waterbury
Clock Company Name: Waterbury Clock
Company
Current Occupant(s): Belco 5th
floor
Radiological Parameter (units) | Location | Measurement Description | Maximum Level | Background | CL |
Gamma radiation (uR/hr) | Rental area | Direct contact | 800 | 10 | 15 |
Measured at Waist level | 800 | ||||
Alpha activity (dpm/100 cm2) | Rental area | Measurement of Loose Material (Smear) | 247 | NR | 20 |
Beta Gamma activity(dpm/100 cm2) | Rental area | Measurement of Loose Material (Smear) | 516 | NR | 20 |
CL = EPA Cleanup Level
dpm = disintegrations per minute
NR = not reported, background counting rates ranged from
0.2-0.3 cpm for alpha, and 30-50 cpm for beta/gamma.
uR/hr
= Micro Roentgen per hour
Table 12. Town: Waterbury
Clock Company Name: Waterbury Clock
Company
Current Occupant(s): Enterprise
Apartments
Radiological Parameters (units) | Location | Measurement Description | Maximum Level | Background | CL |
Gamma radiation (uR/hr) | 1st floor | Direct contact | 0 | 10 | 15 |
Measured at Waist level | 0 | ||||
2nd floor | Direct contact | 0 | |||
Measured at Waist level | 0 | ||||
3rd floor | Direct contact | 0 | |||
Measured at Waist level | 0 | ||||
4th floor Apt 417 |
Direct contact | 240 | |||
Measured at Waist level | 15 | ||||
5th floor Apt 505 |
Direct contact | 30 | 7 | ||
Measured at Waist level | 12 | ||||
5th floor Apt 507 |
Direct contact | 90 | 10 | ||
Measured at Waist level | 30 | ||||
5th floor Apt 508 |
Direct contact | 28 | 8 | ||
Measured at Waist level | 12 | ||||
5th floor Apt 512 |
Direct contact | 30 | 7 | ||
Measured at Waist level | 15 | ||||
5th floor Apt 513 |
Direct contact | 45 | 8 | ||
Measured at Waist level | 15 | ||||
5th floor Apt 514 |
Direct contact | 100 | 10 | ||
Measured at Waist level | 30 | ||||
5th floor Apt 515 |
Direct contact | 110 | 8 | ||
Measured at Waist level | 20 | ||||
5th floor Apt 516 |
Direct contact | 25 | 12 | ||
Measured at Waist level | 15 | ||||
5th floor Apt 517 |
Direct contact | 120 | 10 | ||
Measured at Waist level | 18 | ||||
5th floor Apt 520 |
Direct contact | 30 | 10 | ||
Measured at Waist level | 15 | ||||
5th floor Apt 525 |
Direct contact | 70 | 8 | ||
Measured at Waist level | 12 | ||||
5th floor Hall |
Direct contact | 800 | 8 | ||
Measured at Waist level | 80 | ||||
Radon-222 (pCi/L) | 4th floor | Not applicable | 1.5 | NR | 4 |
CL = EPA Cleanup Level
NR = not reported
pCi/L = Pico Curries per Liter
uR/hr
= Micro Roentgen per hour
Table 13. Town: Waterbury
Clock Company Name: Waterbury Clock
Company
Current Occupant(s): NOW 3rd
through 5th Floors
Radiological Parameters (units) | Location | Measurement Description | Maximum Level | Background | CL |
Gamma radiation (uR/hr) | 3rd floor | Direct contact | 60 | 10 | 15 |
Measured at Waist level | 18 | ||||
4th floor | Direct contact | 180 | 12 | ||
Measured at Waist level | 35 | ||||
5th floor | Direct contact | 4,000 | 12 | ||
Measured at Waist level | 125 | ||||
Radon-222 (pCi/L) | 3rd floor | Not applicable | 0.8 | NR | 4 |
4th floor | Not applicable | 8.5 |
CL = EPA Cleanup Level
NR = not reported
pCi/L = Pico Curries per Liter
uR/hr
= Micro Roentgen per hour
Table 14. Town: Waterbury
Clock Company Name: Waterbury Clock
Company
Current Occupant(s): Ville Swiss
Automatics Automotive 3rd through 5th Floors
Radiological Parameters (units) | Location | Measurement Description | Maximum Level | Background | CL |
Gamma radiation (uR/hr) | 1st floor | Direct contact | Nd | 15 | |
Measured at Waist level | Nd | ||||
2nd floor | Direct contact | Nd | |||
Measured at Waist level | Nd | ||||
3rd floor | Direct contact | 100 | 20 | ||
Measured at Waist level | 20 | ||||
4th floor | Direct contact | 40 | 20 | ||
Measured at Waist level | 20 | ||||
5th floor | Direct contact | 40 | 13 | ||
Measured at Waist level | 13 | ||||
Radon-222 (pCi/L) | 4th floor | Not applicable | 0.3 | 4 |
CL = EPA Cleanup Level
Nd = none detected
pCi/L = Pico Curries per Liter
uR/hr
= Micro Roentgen per hour
Studies have shown that internal deposition of 226Ra results in the induction of skeletal tumors and paranasal sinus carcinomas (cancer of the sinus cavities) (3, 4). Argonne National Laboratory and its' Center for Human Radiobiology have studied the human health effects of radium deposition for over 20 years. Stebbings, et al. (5) reported that in U.S. white females employed as dial painters, the rates of liver, pancreatic, cervical, and uterine cancers were not related to radium exposure. Some cancers of the digestive system, however, may have been indirectly related to radium exposure. They reported that although, there was an increase in multiple myeloma (a form of leukemia), indications were that this increase was related more to the length of employment as a dial painter than the amount of radium in the body. This indirectly suggests the myeloma may be due to the external exposure to the gamma radiation emitted during the radioactive decay of 226Ra.
The major health effects resulting from internally deposited 226Ra are noted in cases dealing with occupational exposure, the majority being radium dial painters. The alpha particle is the major type of damaging radiation from internalized (inhaled or ingested) 226Ra. This decay particle travels very short distances within the body and the majority, if not all its energy is absorbed within the body part where the 226Ra is deposited. 226Ra has chemical characteristics similar to calcium therefore, most of the ingested 226Ra deposits in bones where the greatest exposure and dose is delivered to bone surfaces and perhaps the blood-forming bone marrow. Additionally, more specific information regarding 226Ra is given in Appendix A.
As of 1984, almost 6,000 individuals with all types of exposure to radium had been located
throughout the United States (6). Of the 6,000 identified, 1,907 dial painters were located and had
their radium body burden measured. In this group, there were 44 cases of bone tumors and 19 cases
of sinus or mastoid (associated with the head) carcinomas. These totals include three individuals with
both types of illnesses. The study concluded that these illnesses and skeletal tissue deterioration were
nevertheless unquestionably related to the presence of internal radium.
Radiation doses and related information: International and National
The National Council on Radiation Protection and Measurements (NCRP) is a non-governmental body that makes recommendations to the radiation protection community within the United States. In 1987, the NCRP recommended that in the case of continuous or frequent exposure to radiation, a population should not exceed 1 milliSieverts (mSv; 100 milliRem per year [mRem/yr]) above background. For a population infrequently exposed, a limit of 5 mSv (500 mRem/yr) was recommended (7). In 1994, the NCRP reaffirmed and refined these exposure limits (8).
The radiation protection industry has adopted stringent, acceptable levels of surface contamination that is fixed in place (non-removable) or that which can be removed from the contaminated surface. In the case of removable contamination, these levels are determined by taking a surface smear from a square meter area and averaging the results per 100 square centimeters (cm2). The radioactive material collected by this procedure is analyzed for the specific radionuclide. For non-removable 226Ra, the average allowable limit is 100 dpm per 100 cm2, and the maximum allowable limit in any 100 cm2 area is 300 dpm. If more than 20 dpm can be removed, then the contaminated surface exceeds these federal standards (9).
The US Environmental Protection Agency (EPA) uses Applicable or Relevant and Appropriate Requirements (ARAR) which, in many cases, serve as the determining factor for site cleanup. Because the contamination in these non-Superfund facilities are not specifically addressed by ARAR values, the EPA can set site specific cleanup levels. In 1997 EPA issued OSWER Directive 9200.4-18. Establishment of cleanup levels for Superfund sites with radioactive contamination (10). This directive provides guidance for establishing protective cleanup levels for radioactive contamination at superfund sites. Using this directive, an effective dose of 0.15 milliSieverts (mSv; 15 mRem/yr) equates to an increased lifetime cancer risk of 3 in 10,000, serving as the upper bounds of EPA acceptable risk.
Discussion of removable contamination
Removable contamination indicates how easily radiologic contamination might be transferred to humans or other surfaces. This is performed by using a standard size paper swab and gently but firmly rubbing the paper over an area of 100 square centimeters. The paper is then checked for type of radioactivity removed and the results are expressed as disintegrations per minute (dpm) per 100 square centimeters (cm2) of surface. Surface contamination limits have been established for 226Ra (9); the limit for removable 226Ra contamination is 20 dpm/100 cm2.
The following section summarizes the results presented in the tables above. This section describes the results stratified by town and presents an overview of the radiation surveys conducted thus far. Locations that have not been fully characterized (identified previously pending data) are also discussed.
To determine whether occupants, workers, or visitors have been or are being exposed to radiation,
the CT DPH and the ATSDR evaluate the environmental and human exposure and an exposed
population. There are three types of exposures when radium is present:
- gamma ray exposure occurs when people are near the radium;
- radon exposure, occurs when radium decays into radon and is inhaled (breathed); and
- radium dust exposure occurs through inhalation, dermal contact (direct contact with the skin), and
ingestion (through the mouth) of dust.
The pathways analysis consist of: the source of contamination, a point of exposure, a route of exposure, and an exposed population. The ATSDR categorizes exposure pathways as either completed or potential pathways. For an exposure pathway to be completed all elements of the pathway must be present. Potential pathways are those where there is not sufficient evidence to show that all the elements are present now, could be present in the future, or were present in the past.
Completed exposures have occurred to gamma ray and radon exposure to radium and radon. There is insufficient information to determine whether dust containing radium is present in the air of the affected buildings. In addition, there is insufficient information regarding current or past exposures to dust on any surface in the affected buildings. Consequently, the exposure pathway involving dust is considered potential.
Public Health Implications
Occupants of buildings identified with radium radiation levels above 15 mRem/yr may be at a low
increased risk of developing bone cancer. This risk may be characterized as higher at locations where
the radiation source has been identified as moveable (smearable). These locations may be exposing
occupants to an additional health risk due to inhalation and incidental ingestion of radium-contaminated dust particles. Additionally, elevated levels of radon gas were detected in the 4th floor
of the Waterbury Clock Company building which now houses Belco. This concentration of radon
gas may increase the risk of developing lung cancer among occupants of that facility. The source of
the radon gas is from the radiation decay products of 226Ra.
Recommendations (continued)
Town | Clock Company | Current Occupant | Floor Location | |
Bristol | Sessions Clock Company | DABKO CO | 4th floor* | Building A |
3rd floor* | Building D | |||
Bristol Instrument Gears | 1st floor* | |||
New Haven | New Haven Clock Company | Goodies Repair | 1st floor* | |
Thomaston | Seth Thomas Clock Company | Various Companies | 1st floor* | |
2nd floor* | ||||
3rd floor* | ||||
4th floor* | ||||
Waterbury | Lux Clock Company | Anchor Advanced Products | 1st floor* | |
2nd floor* | ||||
3rd floor* | ||||
4th floor* | ||||
Benrus Clock Company | Bender Plumbing | 4th floor* | ||
5th floor* | ||||
7th floor* | ||||
Waterbury Clock Company | Belco | 2nd floor* | Cutting Room | |
Machine Room | ||||
3rd floor* | Hallway | |||
Store room | ||||
Liba room | ||||
4th floor* | Store room | |||
5th floor* | Rental area | |||
Enterprise Apartments | 4th floor* | Apt 417 | ||
5th floor* | Apt 505 ** | |||
Apt 507 | ||||
Apt 508 | ||||
Apt 512 | ||||
Apt 513 | ||||
Apt 514 | ||||
Apt 515 | ||||
Apt 516 | ||||
Apt 517 | ||||
Apt 520 | ||||
Apt 525 ** | ||||
Hall | ||||
New Opportunities for Waterbury | 3rd floor* | |||
4th floor* | ||||
5th floor* | ||||
Ville Swiss Automatics Automotive | 3rd floor* | |||
4th floor* | ||||
5th floor* |
* Only isolated areas of the floors listed were affected.
** These apartments were slightly below the EPA risk-based cleanup levels at
waist level, but exceeded this value on direct contact.
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